NHC-Based Iron Sensitizers for DSSCs
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NHC-Based Iron Sensitizers for DSSCs

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NHC-Based Iron Sensitizers for DSSCs

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dc.contributor.author Duchanois, Thibaut
dc.contributor.author Liu, Li
dc.contributor.author Pastore, Mariachiara
dc.contributor.author Monari, Antonio
dc.contributor.author Cebrián, Cristina
dc.contributor.author Trolez, Yann
dc.contributor.author Darari, Mohamed
dc.contributor.author Magra, Kevin
dc.contributor.author Francés Monerris, Antonio
dc.contributor.author Domenichini, Edoardo
dc.contributor.author Beley, Marc
dc.contributor.author Assfeld, Xavier
dc.contributor.author Haacke, Stefan
dc.contributor.author Gros, Philippe C.
dc.date.accessioned 2018-10-08T13:45:38Z
dc.date.available 2018-10-08T13:45:38Z
dc.date.issued 2018
dc.identifier.uri http://hdl.handle.net/10550/67734
dc.description.abstract Nanostructured dye-sensitized solar cells (DSSCs) are promising photovoltaic devices because of their low cost and transparency. Ruthenium polypyridine complexes have long been considered as lead sensitizers for DSSCs, allowing them to reach up to 11% conversion efficiency. However, ruthenium suffers from serious drawbacks potentially limiting its widespread applicability, mainly related to its potential toxicity and scarcity. This has motivated continuous research efforts to develop valuable alternatives from cheap earth-abundant metals, and among them, iron is particularly attractive. Making iron complexes applicable in DSSCs is highly challenging due to an ultrafast deactivation of the metal-ligand charge-transfer (MLCT) states into metal-centered (MC) states, leading to inefficient injection into TiO2. In this review, we present our latest developments in the field using Fe(II)-based photosensitizers bearing N-heterocyclic carbene (NHC) ligands, and their use in DSSCs. Special attention is paid to synthesis, photophysical, electrochemical, and computational characterization.
dc.language.iso eng
dc.relation.ispartof Inorganics (Basel), 2018, vol. 6, num. 2, p. 63
dc.rights.uri info:eu-repo/semantics/openAccess
dc.source Duchanois, Thibaut Liu, Li Pastore, Mariachiara Monari, Antonio Cebrián, Cristina Trolez, Yann Darari, Mohamed Magra, Kevin Francés Monerris, Antonio Domenichini, Edoardo Beley, Marc Assfeld, Xavier Haacke, Stefan Gros, Philippe C. 2018 NHC-Based Iron Sensitizers for DSSCs Inorganics (Basel) 6 2 63
dc.subject Ferro
dc.subject Cèl·lules fotoelèctriques
dc.title NHC-Based Iron Sensitizers for DSSCs
dc.type info:eu-repo/semantics/article
dc.date.updated 2018-10-08T13:45:38Z
dc.identifier.doi https://doi.org/10.3390/inorganics6020063
dc.identifier.idgrec 127140

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